Carrier transport characteristics of TIPS-pentacene single crystalline film were controlled by changing the deposition condition of the blade-coating method. Anisotropic carrier transport in the single crystalline grain was visualized by means of the time-resolved microscopic optical second harmonic generation (TRM-SHG) measurement. Slow deposition yields the film with high mobility and large transport anisotropy. For molecular crystals, intermolecular interaction can be modified easily by changing the process condition.